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AI algorithms for gamma-ray spectrometry used in field measurement

Figure 1 : Spectral deformation of a Ba-133 source placed at the center of a steel sphere, as a function of sphere thickness (Geant4 simulations).
In gamma spectrometry, the demand for automated algorithms for
rapid decision-making in low-statistics in situ measurements is high. However, speed is not the only consideration. Algorithms must
also be compatible with detectors with low energy resolution, and
false alerts must be managed robustly, especially if the spectrum is distorted.

CEA-Leti combined machine learning and statistical techniques in SEMSUN, a hybrid spectral demixing algorithm. An interpolation autoencoder (IAE) was used to learn spectral distortions induced by Compton attenuation and scattering phenomena in the source’s environment. The autoencoder, a neural network, can extract the characteristics of a spectrum in a compressed representation (encoder) and can be used as a generative model to reconstruct the spectra from the learned characteristics (decoder). The spectral unmixing technique is based on a mixing model of spectral signatures specific to each radionuclide present. SEMSUN uses the IAE model to impose a constraint on the deformation of these spectral signatures in solving an inverse problem. This hybrid approach optimizes
radionuclide identification and counting by explicitly integrating the physical characteristics of a measurement, unlike a state-of-the-art approach that relies on end-to-end learning.

The IAE model training was based on Geant4 code simulations of radiation-matter interactions in a geometric configuration in which a point source is placed at the center of a sphere (steel, lead), with a 3“×3“ NaI(Tl) detector (Figure 1). Spectrum reconstruction results show that the IAE model effectively captures spectral deformation, allowing us to establish the proof of concept[1].

Figure 1 : Spectral deformation of a Ba-133 source placed at
the center of a steel sphere, as a function of sphere
thickness (Geant4 simulations).

 

To automatically identify radionuclides, SEMSUN was combined with a model selection technique based on a likelihood ratio test, resulting in a new algorithm, MoSeVa[2]. A sparsity criterion was applied to the various
spectral signatures grouped together in a library to determine the presence of a radionuclide. Tests were carried out on different natural background radiation mixtures (up to four radionuclides in a library of twelve spectral signatures). Different counts in the spectra were also studied up to a minimum count of 2,500 events (Figure 2).

 

Figure 2 : Natural background spectrum of Co-57, Co-60,
Ba-133 and Cs-137 simulated for a total of 2,500 events.

 

Hybrid spectral unmixing was compared to a state-ofthe- art end-to-end learning method based on convolutional neural networks used as classifiers or for regression applications. The results confirm that hybrid spectral demixing performs better on low-statistics measurements in terms of identification and robustness, with the expected false alert rate. Hybrid spectral demixing also enables more accurate counting beyond low statistics[3]. The GammaBench benchmark (including spectra, evaluation metrics, etc.) can be used to compare the performance of new developments with hybrid spectral demixing.

"Hybrid spectral demixing offers a solution to the problem of low-statistics in situ measurements sensitive to spectral variability.»

Rebecca Cabean

Christophe Bobin

Research Engineer and Senior Expert — CEA-List

Key figure

×10 MORE ACCURATE

Improvement using hybrid
spectral demixing on
quantization compared to
end-to-end methods.

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Use cases, applications, technology transfer

  • In situ environmental measurements following nuclear or radiological accidents involving the release of radionuclides, detection of illicit trafficking of radioactive materials, radiological characterization during nuclear facility remediation and decommissioning, etc.

 

Flagship publications

  • [1] Phan D.T., et al., “A hybrid Machine Learning unmixing method for automatic analysis of gamma-spectra with spectral variability“. Nuclear Inst. and Methods in Physics Research A 1060 (2024) 169028. https://doi.org/10.23919/EUSIPCO63174.2024.10715033
  • [2] Phan D.T., et al., “Automatic identification and quantification of 𝛾-emitting radionuclides with spectral variability using a hybrid Machine Learning unmixing method.” Radiation Physics and Chemistry 232 (2025) 112654. https://doi.org/10.1016/j.radphyschem.2025.112654
  • [3] Phan D.T., et al., “Comparative study of machine learning and statistical methods for automatic identification and quantification in γ-ray spectrometry.” Nuclear Inst. and Methods in Physics Research A 1083 (2026) 171088. https://doi.org/10.48550/arXiv.2508.08306